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|Title:||Cu–Rh redox relay catalysts for synthesis of azaheterocycles via C–H functionalization||Authors:||Chiba, Shunsuke||Issue Date:||2012||Source:||Chiba, S. (2012). Cu–Rh Redox Relay Catalysts for Synthesis of Azaheterocycles via C–H Functionalization. Chemistry Letters, 41(12), 1554-1559.||Series/Report no.:||Chemistry letters||Abstract:||This Highlight Review describes a Cu–Rh bimetallic redox relay catalytic system that enables efficient synthesis of highly substituted isoquinolines and their derivatives from readily available aryl ketoximes or α-arylvinyl azides with internal alkynes via C–H bond functionalization. A preliminary mechanistic investigation revealed that both the Cu and Rh catalysts are prerequisites to achieve the present process, and play their particular roles with synergistic cooperation during the multistep sequence.||URI:||https://hdl.handle.net/10356/96471
|DOI:||http://dx.doi.org/10.1246/cl.2012.1554||Fulltext Permission:||none||Fulltext Availability:||No Fulltext|
|Appears in Collections:||SPMS Journal Articles|
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