dc.contributor.authorWang, Lu
dc.contributor.authorAmbrosi, Adriano
dc.contributor.authorPumera, Martin
dc.date.accessioned2014-03-17T06:36:29Z
dc.date.available2014-03-17T06:36:29Z
dc.date.copyright2013en_US
dc.date.issued2013
dc.identifier.citationWang, L., Ambrosi, A., & Pumera, M. (2013). “Metal-Free” Catalytic Oxygen Reduction Reaction on Heteroatom-Doped Graphene is Caused by Trace Metal Impurities. Angewandte Chemie International Edition, 52(51), 13818-13821.en_US
dc.identifier.issn1433-7851en_US
dc.identifier.urihttp://hdl.handle.net/10220/18915
dc.description.abstractThe oxygen reduction reaction (ORR) is of high industrial importance. There is a large body of literature showing that metal-based catalytic nanoparticles (e.g. Co, Mn, Fe or hybrid Mn/Co-based nanoparticles) supported on graphene act as efficient catalysts for the ORR. A significant research effort is also directed to the so-called “metal-free” oxygen reduction reaction on heteroatom-doped graphene surfaces. While such studies of the ORR on nonmetallic heteroatom-doped graphene are advertised as “metal-free” there is typically no sufficient effort to characterize the doped materials to verify that they are indeed free of any trace metal. Here we argue that the claimed “metal-free” electrocatalysis of the oxygen reduction reaction on heteroatom-doped graphene is caused by metallic impurities present within the graphene materials.en_US
dc.language.isoenen_US
dc.relation.ispartofseriesAngewandte chemie international editionen_US
dc.rights© 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.en_US
dc.subjectDRNTU::Engineering::Materials::Nanostructured materials
dc.title“Metal-free” catalytic oxygen reduction reaction on heteroatom-doped graphene is caused by trace metal impuritiesen_US
dc.typeJournal Article
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen_US
dc.identifier.doihttp://dx.doi.org/10.1002/anie.201309171


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