dc.contributor.authorChen, Mengli
dc.contributor.authorGoodkin, Nathalie Fairbank
dc.contributor.authorBoyle, Edward A.
dc.contributor.authorSwitzer, Adam Douglas
dc.contributor.authorBolton, Annette
dc.date.accessioned2016-09-22T05:51:37Z
dc.date.available2016-09-22T05:51:37Z
dc.date.issued2016
dc.identifier.citationChen, M., Goodkin, N. F., Boyle, E. A., Switzer, A. D., & Bolton, A. (2016). Lead in the western South China Sea: Evidence of atmospheric deposition and upwelling. Geophysical Research Letters, 43(9), 4490-4499.en_US
dc.identifier.issn0094-8276en_US
dc.identifier.urihttp://hdl.handle.net/10220/41473
dc.description.abstractIn recent decades, rapid industrial developments have increased lead (Pb) inputs to the South China Sea. To quantify the increasing variability, we investigated 170 years of skeletal Pb and Pb isotopes from an offshore, central Vietnamese coral. The Pb/Ca in the coral was 10–16 nmol/mol before the mid-1950s and increased to more than 30 nmol/mol by 2000. While the regional phaseout of leaded petrol commenced in 2000, coral Pb/Ca continued increasing until 2004, possibly due to regional upwelling and the transport of previously emitted Pb from tropical Pacific waters. The 206Pb/207Pb ratio in the coral was 1.191–1.195 before mid-1950s, suggesting natural sources. Since then, the ratio decreased, reaching ~1.165 in 2004. Lead isotopes show high linearity between natural and Chinese emitted Pb, with the latter contributing ~40%~60% of the skeletal Pb after 2000.en_US
dc.description.sponsorshipNRF (Natl Research Foundation, S’pore)en_US
dc.description.sponsorshipMOE (Min. of Education, S’pore)en_US
dc.format.extent10 p.en_US
dc.language.isoenen_US
dc.relation.ispartofseriesGeophysical Research Lettersen_US
dc.rights©2016 The Authors. This is an open access article under the terms of the Creative Commons Attribution-NonCommercial-NoDerivs License, which permits use and distribution in any medium, provided the original work is properly cited, the use is non-commercial and no modifications or adaptations are made.en_US
dc.subjectPb isotopesen_US
dc.subjectcoralen_US
dc.titleLead in the western South China Sea: Evidence of atmospheric deposition and upwellingen_US
dc.typeJournal Article
dc.contributor.researchEarth Observatory of Singapore
dc.contributor.schoolAsian School of the Environment
dc.identifier.doihttp://dx.doi.org/10.1002/2016GL068697
dc.description.versionPublished versionen_US


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