dc.contributor.authorZhang, Qing
dc.contributor.authorSu, Rui
dc.contributor.authorLiu, Xinfeng
dc.contributor.authorXing, Jun
dc.contributor.authorSum, Tze Chien
dc.contributor.authorXiong, Qihua
dc.date.accessioned2017-08-07T03:32:15Z
dc.date.available2017-08-07T03:32:15Z
dc.date.issued2016
dc.identifier.citationZhang, Q., Su, R., Liu, X., Xing, J., Sum, T. C., & Xiong, Q. (2016). High-Quality Whispering-Gallery-Mode Lasing from Cesium Lead Halide Perovskite Nanoplatelets. Advanced Functional Materials, 26(34), 6238-6245.en_US
dc.identifier.issn1616-301Xen_US
dc.identifier.urihttp://hdl.handle.net/10220/43556
dc.description.abstractSemiconductor micro/nano-cavities with high quality factor (Q) and small modal volume provide critical platforms for exploring strong light-matter interactions and quantum optics, enabling further development of coherent and quantum photonic devices. Constrained by exciton binding energy and thermal fluctuation, only a handful of wide-band semiconductors such as ZnO and GaN have stable excitons at room temperature. Metal halide perovskite with cubic lattice and well-controlled exciton may provide solutions. In this work, high-quality single-crystalline cesium lead halide CsPbX3 (X = Cl, Br, I) whispering-gallery-mode (WGM) microcavities are synthesized by vapor-phase van der Waals epitaxy method. The as-grown perovskites show strong emission and stable exciton at room temperature over the whole visible spectra range. By varying the halide composition, multi-color (400–700 nm).WGM excitonic lasing is achieved at room temperature with low threshold (~ 2.0 μJ cm−2) and high spectra coherence (~0.14–0.15 nm). The results advocate the promise of inorganic perovskites towards development of optoelectronic devices and strong light-matter coupling in quantum optics.en_US
dc.description.sponsorshipNRF (Natl Research Foundation, S’pore)en_US
dc.description.sponsorshipMOE (Min. of Education, S’pore)en_US
dc.format.extent21 p.en_US
dc.language.isoenen_US
dc.relation.ispartofseriesAdvanced Functional Materialsen_US
dc.rights© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This is the author created version of a work that has been peer reviewed and accepted for publication by Advanced Functional Materials, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [http://dx.doi.org/10.1002/adfm.201601690].en_US
dc.subjectCesium Lead Halideen_US
dc.subjectPerovskiteen_US
dc.titleHigh-Quality Whispering-Gallery-Mode Lasing from Cesium Lead Halide Perovskite Nanoplateletsen_US
dc.typeJournal Article
dc.contributor.researchEnergy Research Institute @NTUen_US
dc.contributor.schoolSchool of Electrical and Electronic Engineeringen_US
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen_US
dc.identifier.doihttp://dx.doi.org/10.1002/adfm.201601690
dc.description.versionAccepted versionen_US
dc.contributor.organizationNOVITAS, Nanoelectronics Centre of Excellenceen_US


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