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https://hdl.handle.net/10356/105224
Title: | Nitrogen-doped graphene-supported transition-metals carbide electrocatalysts for oxygen reduction reaction | Authors: | Chen, Minghua Liu, Jilei Zhou, Weijiang Lin, Jianyi Shen, Zexiang |
Keywords: | DRNTU::Science::Chemistry::Physical chemistry::Catalysis | Issue Date: | 2015 | Source: | Chen, M., Liu, J., Zhou, W., Lin, J., & Shen, Z. (2015). Nitrogen-doped graphene-supported transition-metals carbide electrocatalysts for oxygen reduction reaction. Scientific reports, 5, 10389-. | Series/Report no.: | Scientific reports | Abstract: | A novel and facile two-step strategy has been designed to prepare high performance bi-transition-metals (Fe- and Mo-) carbide supported on nitrogen-doped graphene (FeMo-NG) as electrocatalysts for oxygen reduction reactions (ORR). The as-synthesized FeMo carbide -NG catalysts exhibit excellent electrocatalytic activities for ORR in alkaline solution, with high onset potential (−0.09 V vs. saturated KCl Ag/AgCl), nearly four electron transfer number (nearly 4) and high kinetic-limiting current density (up to 3.5 mA cm−2 at −0.8 V vs. Ag/AgCl). Furthermore, FeMo carbide -NG composites show good cycle stability and much better toxicity tolerance durability than the commercial Pt/C catalyst, paving their application in high-performance fuel cell and lithium-air batteries. | URI: | https://hdl.handle.net/10356/105224 http://hdl.handle.net/10220/25957 |
ISSN: | 2045-2322 | DOI: | 10.1038/srep10389 | Schools: | School of Mechanical and Aerospace Engineering School of Physical and Mathematical Sciences |
Research Centres: | Energy Research Institute @ NTU (ERI@N) | Rights: | This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ | Fulltext Permission: | open | Fulltext Availability: | With Fulltext |
Appears in Collections: | ERI@N Journal Articles MAE Journal Articles SPMS Journal Articles |
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Nitrogen-doped graphene-supported transition-metals carbide electrocatalysts for oxygen reduction reaction.pdf | 1.69 MB | Adobe PDF | View/Open |
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