Please use this identifier to cite or link to this item:
https://hdl.handle.net/10356/106414
Title: | Degenerative xanthate transfer to olefins under visible-light photocatalysis | Authors: | Kaga, Atsushi Wu, Xiangyang Lim, Joel Yi Jie Hayashi, Hirohito Lu, Yunpeng Yeow, Edwin Kok Lee Chiba, Shunsuke |
Keywords: | Energy Transfer Olefin DRNTU::Science::Chemistry |
Issue Date: | 2018 | Source: | Kaga, A., Wu, X., Lim, J. Y. J., Hayashi, H., Lu, Y., Yeow, E. K. L., & Chiba, S. (2018). Degenerative xanthate transfer to olefins under visible-light photocatalysis. Beilstein Journal of Organic Chemistry, 14, 3047-3058. doi:10.3762/bjoc.14.283 | Series/Report no.: | Beilstein Journal of Organic Chemistry | Abstract: | The degenerative transfer of xanthates to olefins is enabled by the iridium-based photocatalyst [Ir{dF(CF3)ppy}2(dtbbpy)](PF6) under blue LED light irradiation. Detailed mechanistic investigations through kinetics and photophysical studies revealed that the process operates under a radical chain mechanism, which is initiated through triplet-sensitization of xanthates by the long-lived triplet state of the iridium-based photocatalyst. | URI: | https://hdl.handle.net/10356/106414 http://hdl.handle.net/10220/47422 |
ISSN: | 1860-5397 | DOI: | 10.3762/bjoc.14.283 | Schools: | School of Physical and Mathematical Sciences | Rights: | © 2018 Kaga et al.; licensee Beilstein-Institut. This is an Open Access article under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0). Please note that the reuse, redistribution and reproduction in particular requires that the authors and source are credited. The license is subject to the Beilstein Journal of Organic Chemistry terms and conditions:(https://www.beilstein-journals.org/bjoc) | Fulltext Permission: | open | Fulltext Availability: | With Fulltext |
Appears in Collections: | SPMS Journal Articles |
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Degenerative xanthate transfer to olefins under visible-light photocatalysis.pdf | 1.67 MB | Adobe PDF | ![]() View/Open |
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