Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/107168
Title: Electroosmotic flow hysteresis for dissimilar ionic solutions
Authors: Lim, An Eng
Lim, Chun Yee
Lam, Yee Cheong
Keywords: DRNTU::Engineering::Mechanical engineering::Fluid mechanics
Issue Date: 2015
Source: Lim, A. E., Lim, C. Y., & Lam, Y. C. (2015). Electroosmotic flow hysteresis for dissimilar ionic solutions. Biomicrofluidics, 9.
Series/Report no.: Biomicrofluidics
Abstract: Electroosmotic flow (EOF) with two or more fluids is commonly encountered in various microfluidics applications. However, no investigation has hitherto been conducted to investigate the hysteretic or flow direction-dependent behavior during the displacement flow of solutions with dissimilar ionic species. In this investigation, electroosmotic displacement flow involving dissimilar ionic solutions was studied experimentally through a current monitoring method and numerically through finite element simulations. The flow hysteresis can be characterized by the turning and displacement times; turning time refers to the abrupt gradient change of current-time curve while displacement time is the time for one solution to completely displace the other solution. Both experimental and simulation results illustrate that the turning and displacement times for a particular solution pair can be directional-dependent, indicating that the flow conditions in the microchannel are not the same in the two different flow directions. The mechanics of EOF hysteresis was elucidated through the theoretical model which includes the ionic mobility of each species, a major governing parameter. Two distinct mechanics have been identified as the causes for the EOF hysteresis involving dissimilar ionic solutions: the widening/sharpening effect of interfacial region between the two solutions and the difference in ion concentration distributions (and thus average zeta potentials) in different flow directions. The outcome of this investigation contributes to the fundamental understanding of flow behavior in microfluidic systems involving solution pair with dissimilar ionic species.
URI: https://hdl.handle.net/10356/107168
http://hdl.handle.net/10220/25458
ISSN: 1932-1058(electronic)
DOI: 10.1063/1.4917386
Rights: © 2015 AIP Publishing LLC. This paper was published in Biomicrofluidics and is made available as an electronic reprint (preprint) with permission of AIP Publishing LLC. The paper can be found at the following official DOI: [http://dx.doi.org/10.1063/1.4917386]. One print or electronic copy may be made for personal use only. Systematic or multiple reproduction, distribution to multiple locations via electronic or other means, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper is prohibited and is subject to penalties under law.
Fulltext Permission: open
Fulltext Availability: With Fulltext
Appears in Collections:MAE Journal Articles

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