Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/138614
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dc.contributor.authorZhang, Huabinen_US
dc.contributor.authorYu, Leen_US
dc.contributor.authorChen, Taoen_US
dc.contributor.authorZhou, Weien_US
dc.contributor.authorLou, David Xiong Wenen_US
dc.date.accessioned2020-05-11T04:24:05Z-
dc.date.available2020-05-11T04:24:05Z-
dc.date.issued2018-
dc.identifier.citationZhang, H., Yu, L., Chen, T., Zhou, W., & Lou, D. X. W. (2018). Surface modulation of hierarchical MoS2 nanosheets by Ni single atoms for enhanced electrocatalytic hydrogen evolution. Advanced Functional Materials, 28(51), 1807086-. doi:10.1002/adfm.201807086en_US
dc.identifier.issn1616-301Xen_US
dc.identifier.urihttps://hdl.handle.net/10356/138614-
dc.description.abstractSurface modulation at the atomic level is an important approach for tuning surface chemistry and boosting the catalytic performance. Here, a surface modulation strategy is demonstrated through the decoration of isolated Ni atoms onto the basal plane of hierarchical MoS2 nanosheets supported on multichannel carbon nanofibers for boosted hydrogen evolution activity. X-ray absorption fine structure investigation and density functional theory (DFT) calculation reveal that the MoS2 surface decorated with isolated Ni atoms displays highly strengthened H binding. Benefiting from the unique tubular structure and basal plane modulation, the newly developed MoS2 catalyst exhibits excellent hydrogen evolution activity and stability. This single-atom modification strategy opens up new avenues for tuning the intrinsic catalytic activity toward electrocatalytic water splitting and other energy-related processes.en_US
dc.description.sponsorshipNRF (Natl Research Foundation, S’pore)en_US
dc.language.isoenen_US
dc.relation.ispartofAdvanced Functional Materialsen_US
dc.rights© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. All rights reserved. This paper was published in Advanced Functional Materials and is made available with permission of WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.en_US
dc.subjectEngineering::Chemical engineeringen_US
dc.titleSurface modulation of hierarchical MoS2 nanosheets by Ni single atoms for enhanced electrocatalytic hydrogen evolutionen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Chemical and Biomedical Engineeringen_US
dc.identifier.doi10.1002/adfm.201807086-
dc.description.versionAccepted versionen_US
dc.identifier.scopus2-s2.0-85055513351-
dc.identifier.issue51en_US
dc.identifier.volume28en_US
dc.subject.keywordsHydrogen Evolution Reactionen_US
dc.subject.keywordsMoS2en_US
item.grantfulltextopen-
item.fulltextWith Fulltext-
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