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Title: N‐type SnSe2 oriented‐nanoplate‐based pellets for high thermoelectric performance
Authors: Luo, Yubo
Zheng, Yun
Luo, Zhongzhen
Hao, Shiqiang
Du, Chengfeng
Liang, Qinghua
Li, Zhong
Khor, Khiam Aik
Hippalgaonkar, Kedar
Xu, Jianwei
Yan, Qingyu
Wolverton, Chris
Kanatzidis, Mercouri G.
Keywords: Engineering::Materials
Issue Date: 2017
Source: Luo, Y., Zheng, Y., Luo, Z., Hao, S., Du, C., Liang, Q., . . . Kanatzidis, M. G. (2018). N‐type SnSe2 oriented‐nanoplate‐based pellets for high thermoelectric performance. Advanced Energy Materials, 8(8), 1702167-. doi:10.1002/aenm.201702167
Journal: Advanced Energy Materials
Abstract: It is reported that electron doped n-type SnSe2 nanoplates show promising thermoelectric performance at medium temperatures. After simultaneous introduction of Se deficiency and Cl doping, the Fermi level of SnSe2 shifts toward the conduction band, resulting in two orders of magnitude increase in carrier concentration and a transition to degenerate transport behavior. In addition, all-scale hierarchical phonon scattering centers, such as point defects, nanograin boundaries, stacking faults, and the layered nanostructures, cooperate to produce very low lattice thermal conductivity. As a result, an enhanced in-plane thermoelectric figure of merit ZTmax of 0.63 is achieved for a 1.5 at% Cl doped SnSe1.95 pellet at 673 K, which is much higher than the corresponding in-plane ZT of pure SnSe2 (0.08).
ISSN: 1614-6832
DOI: 10.1002/aenm.201702167
Rights: © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. All rights reserved.
Fulltext Permission: none
Fulltext Availability: No Fulltext
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