Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/140447
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dc.contributor.authorLee, Junwooen_US
dc.contributor.authorTan, Matthew Wei Mingen_US
dc.contributor.authorParida, Kaushiken_US
dc.contributor.authorThangavel, Gurunathanen_US
dc.contributor.authorPark, Sang Ahen_US
dc.contributor.authorPark, Taihoen_US
dc.contributor.authorLee, Pooi Seeen_US
dc.date.accessioned2020-05-29T03:55:09Z-
dc.date.available2020-05-29T03:55:09Z-
dc.date.issued2019-
dc.identifier.citationLee, J., Tan, M. W. M., Parida, K., Thangavel, G., Park, S. A., Park, T., & Lee, P. S. (2020). Water‐processable, stretchable, self‐healable, thermally stable, and transparent ionic conductors for actuators and sensors. Advanced Materials, 32(7), 1906679-. doi:10.1002/adma.201906679en_US
dc.identifier.issn0935-9648en_US
dc.identifier.urihttps://hdl.handle.net/10356/140447-
dc.description.abstractFor emerging biocompatible, wearable, and stretchable epidermal electronic devices, it is essential to realize novel stretchable conductors with the attributes of transparency, low‐cost and nontoxic components, green‐solvent processbility, self‐healing, and thermal stabililty. Although conducting materials–rubber composites, ionic hydrogels, organogels have been developed, no stretchable material system that meets all the outlined requirements has been reported. Here, a series of P(SPMA‐r‐MMA) polymers with different ratios of ionic side chains is designed and synthesized, and it is demonstrated that the resulting stretchable ionic conductors with glycerol are transparent, water processable, self‐healable, and thermally stable due to the chemically linked ionic side chain, satisfying all of the aforementioned requirements. Among the series of polymer gels, the P(SPMA0.75‐r‐MMA0.25) gel shows optimum conductivity (6.7 × 10−4 S cm−1), stretchability (2636% of break at elongation), and self‐healing (98.3% in 3 h) properties. Accordingly, the transparent and self‐healable P(SPMA0.75‐r‐MMA0.25) gels are used to realize thermally robust actuators up to 100 °C and deformable and self‐healable thermal sensors.en_US
dc.description.sponsorshipNational Research Foundation (NRF)en_US
dc.language.isoenen_US
dc.relationNRF-CRP13-2014-02en_US
dc.relationNRF-NRFI2016-05en_US
dc.relationNRF-2012M3A6A5055225en_US
dc.relation.ispartofAdvanced Materialsen_US
dc.rightsThis is the accepted version of the following article: Lee, J., Tan, M. W. M., Parida, K., Thangavel, G., Park, S. A., Park, T., & Lee, P. S. (2020). Water‐processable, stretchable, self‐healable, thermally stable, and transparent ionic conductors for actuators and sensors. Advanced Materials, 32(7), 1906679-, which has been published in final form at https://doi.org/10.1002/adma.201906679. This article may be used for non-commercial purposes in accordance with the Wiley Self-Archiving Policy [https://authorservices.wiley.com/authorresources/Journal-Authors/licensing/self-archiving.html].en_US
dc.subjectScience::Chemistryen_US
dc.titleWater‐processable, stretchable, self‐healable, thermally stable, and transparent ionic conductors for actuators and sensorsen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Materials Science & Engineeringen_US
dc.identifier.doi10.1002/adma.201906679-
dc.description.versionAccepted versionen_US
dc.identifier.issue7en_US
dc.identifier.volume32en_US
dc.subject.keywordsActuatorsen_US
dc.subject.keywordsIonic Conductorsen_US
dc.description.acknowledgementThis research is partially supported by grants from the National Research Foundation, Prime Minister’s Office, Singapore under its Campus of Research Excellence and Technological Enterprise (CREATE) programme, the Competitive Research Programme (Award No. NRF-CRP13-2014-02), the NRF Investigatorship (Award No. NRF-NRFI2016-05), the Center for Advanced Soft Electronics under the Global Frontier Research Program (Code No. NRF-2012M3A6A5055225), and the National Research Foundation of Korea (NRF) grant (Code No. 2018R1A2A1A05079144) funded by the Korea government (MSIP).en_US
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