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|Title:||Water in rechargeable multivalent‐ion batteries : an electrochemical Pandora's box||Authors:||Manalastas, William, Jr.
|Keywords:||Engineering::Materials||Issue Date:||2018||Source:||Manalastas, W., Jr., Kumar, S., Verma, V., Zhang, L., Yuan, D., & Srinivasan, M. (2019). Water in rechargeable multivalent‐ion batteries : an electrochemical Pandora's box. ChemSusChem, 12(2), 379-396. doi:10.1002/cssc.201801523||Project:||NRF2017-08/NRF2016NRF-NRFI001-22||Journal:||ChemSusChem||Abstract:||Multivalent‐ion batteries built on water‐based electrolytes represent energy storage at suitable price points, competitive performance, and enhanced safety. However, to comply with modern energy‐density requirements, the battery must be reversible within an operating voltage window greater than 1.23 V or the electrochemical stability limits of free water. Taking advantage of its powerful solvation and catalytic activities, adding water to electrolyte preparations can unlock a wider gamut of liquid mixtures compared with strictly nonaqueous systems. However, a point‐by‐point sweep of all potential formulations is arduous and ineffective without some form of systematic rationalization. The present Review consolidates recent progress, pitfalls, limits, and insights critical to expediting aqueous electrolyte designs to boost multivalent‐ion battery outputs.||URI:||https://hdl.handle.net/10356/140527||ISSN:||1864-5631||DOI:||10.1002/cssc.201801523||Rights:||This is the accepted version of the following article: Manalastas, W., Jr., Kumar, S., Verma, V., Zhang, L., Yuan, D., & Srinivasan, M. (2019). Water in rechargeable multivalent‐ion batteries : an electrochemical Pandora's box. ChemSusChem, 12(2), 379-396. doi:10.1002/cssc.201801523, which has been published in final form at https://doi.org/10.1002/cssc.201801523. This article may be used for non-commercial purposes in accordance with the Wiley Self-Archiving Policy [https://authorservices.wiley.com/authorresources/Journal-Authors/licensing/self-archiving.html].||Fulltext Permission:||open||Fulltext Availability:||With Fulltext|
|Appears in Collections:||MSE Journal Articles|
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