Please use this identifier to cite or link to this item:
https://hdl.handle.net/10356/142141
Title: | Vertical silver@silver chloride core-shell nanowire array for carbon dioxide electroreduction | Authors: | Ge, Junyu Long, Jun Sun, Zixu Feng, Han Hu, Jie Koh, See Wee Yu, Qing Xiao, Jianping Li, Hong |
Keywords: | Engineering::Electrical and electronic engineering | Issue Date: | 2019 | Source: | Ge, J., Long, J., Sun, Z., Feng, H., Hu, J., Koh, S. W., . . . Li, H. (2019). Vertical silver@silver chloride core-shell nanowire array for carbon dioxide electroreduction. ACS Applied Energy Materials, 2(9), 6163-6169. doi:10.1021/acsaem.9b01286 | Journal: | ACS Applied Energy Materials | Abstract: | Core-shell nanowires with conductive metal cores and active catalyst shells hold great promise for making a catalyst electrode with high total activity. Indeed, core-shell nanowire arrays have been demonstrated as the catalyst in various electrochemical reactions, yet their catalytic roles are underexplored for carbon dioxide (CO2) electroreduction. Herein, we report a reduced silver@silver chloride (Ag@AgClx) core-shell nanowire array for electrocatalytic CO2 reduction. The Ag@AgClx core-shell array electrode shows high total activity including low onset potential and high current density. The strong electronic coupling between AgClx and the Ag core results in the record-high specific CO2RR activity to date. | URI: | https://hdl.handle.net/10356/142141 | ISSN: | 2574-0962 | DOI: | 10.1021/acsaem.9b01286 | Schools: | School of Electrical and Electronic Engineering School of Mechanical and Aerospace Engineering |
Organisations: | Advanced Environmental Biotechnology Centre Centre for Micro-/Nano-electronics (NOVITAS) CINTRA CNRS/NTU/THALES |
Research Centres: | Nanyang Environment and Water Research Institute | Rights: | This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Energy Materials, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acsaem.9b01286 | Fulltext Permission: | open | Fulltext Availability: | With Fulltext |
Appears in Collections: | MAE Journal Articles |
Files in This Item:
File | Description | Size | Format | |
---|---|---|---|---|
Vertical Silver Chloride-Silver Core-Shell Nanowire Array for Carbon Dioxide Electroreduction-Final.pdf | 803.78 kB | Adobe PDF | View/Open | |
Vertical Silver Chloride-Silver Core-Shell Nanowire Array for Carbon Dioxide Electroreduction Supporting Information_Final.pdf | 1.34 MB | Adobe PDF | View/Open |
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