Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/153153
Full metadata record
DC FieldValueLanguage
dc.contributor.authorZhao, Huen_US
dc.contributor.authorLu, Danen_US
dc.contributor.authorWang, Jiaruien_US
dc.contributor.authorTu, Wengguangen_US
dc.contributor.authorWu, Danen_US
dc.contributor.authorKoh, See Weeen_US
dc.contributor.authorGao, Pingqien_US
dc.contributor.authorXu, Zhichuan Jasonen_US
dc.contributor.authorDeng, Silien_US
dc.contributor.authorZhou, Yanen_US
dc.contributor.authorYou, Boen_US
dc.contributor.authorLi, Hongen_US
dc.date.accessioned2021-11-12T05:11:03Z-
dc.date.available2021-11-12T05:11:03Z-
dc.date.issued2021-
dc.identifier.citationZhao, H., Lu, D., Wang, J., Tu, W., Wu, D., Koh, S. W., Gao, P., Xu, Z. J., Deng, S., Zhou, Y., You, B. & Li, H. (2021). Raw biomass electroreforming coupled to green hydrogen generation. Nature Communications, 12, 2008-. https://dx.doi.org/10.1038/s41467-021-22250-9en_US
dc.identifier.issn2041-1723en_US
dc.identifier.urihttps://hdl.handle.net/10356/153153-
dc.description.abstractDespite the tremendous progress of coupling organic electrooxidation with hydrogen generation in a hybrid electrolysis, electroreforming of raw biomass coupled to green hydrogen generation has not been reported yet due to the rigid polymeric structures of raw biomass. Herein, we electrooxidize the most abundant natural amino biopolymer chitin to acetate with over 90% yield in hybrid electrolysis. The overall energy consumption of electrolysis can be reduced by 15% due to the thermodynamically and kinetically more favorable chitin oxidation over water oxidation. In obvious contrast to small organics as the anodic reactant, the abundance of chitin endows the new oxidation reaction excellent scalability. A solar-driven electroreforming of chitin and chitin-containing shrimp shell waste is coupled to safe green hydrogen production thanks to the liquid anodic product and suppression of oxygen evolution. Our work thus demonstrates a scalable and safe process for resource upcycling and green hydrogen production for a sustainable energy future.en_US
dc.description.sponsorshipAgency for Science, Technology and Research (A*STAR)en_US
dc.description.sponsorshipMinistry of Education (MOE)en_US
dc.description.sponsorshipNanyang Technological Universityen_US
dc.language.isoenen_US
dc.relationM408050000en_US
dc.relation2018-T1-001-051en_US
dc.relationA1983c0029en_US
dc.relation.ispartofNature Communicationsen_US
dc.rights© 2021 The Author(s). This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/ licenses/by/4.0/.en_US
dc.subjectEngineering::Chemical engineering::Chemical processesen_US
dc.subjectEngineering::Chemical engineering::Fuelen_US
dc.titleRaw biomass electroreforming coupled to green hydrogen generationen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Mechanical and Aerospace Engineeringen_US
dc.contributor.schoolSchool of Materials Science and Engineeringen_US
dc.contributor.schoolSchool of Civil and Environmental Engineeringen_US
dc.contributor.schoolSchool of Electrical and Electronic Engineeringen_US
dc.contributor.researchAdvanced Environmental Biotechnology Centre (AEBC)en_US
dc.contributor.researchNanyang Environment and Water Research Instituteen_US
dc.contributor.researchCentre for Micro-/Nano-electronics (NOVITAS)en_US
dc.contributor.researchCNRS International NTU THALES Research Alliancesen_US
dc.identifier.doi10.1038/s41467-021-22250-9-
dc.description.versionPublished versionen_US
dc.identifier.volume12en_US
dc.identifier.spage2008en_US
dc.subject.keywordsChemical Engineeringen_US
dc.subject.keywordsElectrocatalysisen_US
dc.description.acknowledgementThis work was supported by Nanyang Technological University under NAP award (M408050000), Singapore Ministry of Education Tier 1 program (2018-T1-001-051), and A*STAR Science & Engineering Research Council AME IRG funding (A1983c0029).en_US
item.grantfulltextopen-
item.fulltextWith Fulltext-
Appears in Collections:CEE Journal Articles
EEE Journal Articles
MAE Journal Articles
MSE Journal Articles
NEWRI Journal Articles
Files in This Item:
File Description SizeFormat 
s41467-021-22250-9 (1).pdfpublished version6.69 MBAdobe PDFThumbnail
View/Open

SCOPUSTM   
Citations 10

42
Updated on Oct 2, 2022

Web of ScienceTM
Citations 10

40
Updated on Oct 1, 2022

Page view(s)

149
Updated on Oct 6, 2022

Download(s) 50

44
Updated on Oct 6, 2022

Google ScholarTM

Check

Altmetric


Plumx

Items in DR-NTU are protected by copyright, with all rights reserved, unless otherwise indicated.