Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/163084
Full metadata record
DC FieldValueLanguage
dc.contributor.authorTeh, Yee Wenen_US
dc.contributor.authorEr, Chen-Chenen_US
dc.contributor.authorKong, Xin Yingen_US
dc.contributor.authorNg, Boon-Junnen_US
dc.contributor.authorYong, Siek-Tingen_US
dc.contributor.authorChai, Siang-Piaoen_US
dc.date.accessioned2022-11-21T03:57:39Z-
dc.date.available2022-11-21T03:57:39Z-
dc.date.issued2022-
dc.identifier.citationTeh, Y. W., Er, C., Kong, X. Y., Ng, B., Yong, S. & Chai, S. (2022). Charge modulation at atomic-level through substitutional sulfur doping into atomically thin Bi₂ WO₆ toward promoting photocatalytic CO₂ reduction. ChemSusChem, 15(14), e202200471-. https://dx.doi.org/10.1002/cssc.202200471en_US
dc.identifier.issn1864-5631en_US
dc.identifier.urihttps://hdl.handle.net/10356/163084-
dc.description.abstractPhotocatalytic reduction of CO2 has attracted enormous interest as a sustainable and renewable source of energy. In the past decade, numerous bulk-type semiconductors have been developed, but the existing designs suffer many limitations, namely rapid recombination of charge carriers and weak light absorption ability. Herein, a bottom-up approach was developed to design atomically thin sulfur-doped Bi2 WO6 perovskite nanosheets (S-BWO) with improved reduction ability, extended visible light absorption, prolonged lifetime of charge carriers, enhanced adsorption of CO2 , and reduced work function. Compared with pristine Bi2 WO6 (P-BWO), S-BWO nanosheets exhibited a 3-fold improvement in photocatalytic reduction of CO2 under simulated sunlight irradiation. Experimental studies and density functional theory calculations revealed the synergistic roles of atomically thin nanosheets and S atoms in promoting photocatalytic efficiency.en_US
dc.language.isoenen_US
dc.relation.ispartofChemSusChemen_US
dc.rights© 2022 The Authors. ChemSusChem published by Wiley-VCH GmbH. This is an open access article under the terms of the Creative Commons Attribution Non-Commercial License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes.en_US
dc.subjectScience::Chemistryen_US
dc.titleCharge modulation at atomic-level through substitutional sulfur doping into atomically thin Bi₂ WO₆ toward promoting photocatalytic CO₂ reductionen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen_US
dc.identifier.doi10.1002/cssc.202200471-
dc.description.versionPublished versionen_US
dc.identifier.pmid35447013-
dc.identifier.scopus2-s2.0-85130344354-
dc.identifier.issue14en_US
dc.identifier.volume15en_US
dc.identifier.spagee202200471en_US
dc.subject.keywordsDensity Functional Theoryen_US
dc.subject.keywordsNanosheetsen_US
dc.description.acknowledgementThis work was funded by the Ministry of Higher Education (MOHE) Malaysia under the Fundamental Research Grant Scheme (FRGS). Project Number: FRGS/1/2019/TK02/MUSM/01/1. Open access publishing facilitated by Monash University, as part of the Wiley-Monash University agreement via the Council of Australian University Librarians.en_US
item.grantfulltextopen-
item.fulltextWith Fulltext-
Appears in Collections:SPMS Journal Articles

SCOPUSTM   
Citations 50

5
Updated on Jan 28, 2023

Web of ScienceTM
Citations 50

4
Updated on Jan 28, 2023

Page view(s)

21
Updated on Feb 3, 2023

Download(s)

5
Updated on Feb 3, 2023

Google ScholarTM

Check

Altmetric


Plumx

Items in DR-NTU are protected by copyright, with all rights reserved, unless otherwise indicated.