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dc.contributor.authorWu, Binen_US
dc.contributor.authorMeng, Haibingen_US
dc.contributor.authorMorales, Dulce M.en_US
dc.contributor.authorZeng, Fengen_US
dc.contributor.authorZhu, Junjiangen_US
dc.contributor.authorWang, Baoen_US
dc.contributor.authorRisch, Marcelen_US
dc.contributor.authorXu, Jason Zhichuanen_US
dc.contributor.authorPetit, Tristanen_US
dc.identifier.citationWu, B., Meng, H., Morales, D. M., Zeng, F., Zhu, J., Wang, B., Risch, M., Xu, J. Z. & Petit, T. (2022). Nitrogen-rich carbonaceous materials for advanced oxygen electrocatalysis: synthesis, characterization, and activity of nitrogen sites. Advanced Functional Materials, 32(31), 2204137-.
dc.description.abstractNitrogen-doped carbons are among the fastest-growing class of materials used for oxygen electrocatalysis, namely, the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER), thanks to their low cost, environmental friendliness, excellent electrical conductivity, and scalable synthesis. The perspective of replacing precious metal-based electrocatalysts with nitrogen-doped carbon is highly desirable for reducing costs in energy conversion and storage systems. In this review, the role of nitrogen and N-induced structural defects on the enhanced performance of N-doped carbon electrocatalysts toward the OER and the ORR as well as their applications for energy conversion and storage technologies is summarized. The synthesis of N-doped carbon electrocatalysts and the characterization of their nitrogen functional groups and active sites for the conversion of oxygen are also reviewed. The electrocatalytic performance of the main types of N-doped carbon materials for OER/ORR electrocatalysis are then discussed. Finally, major challenges and future opportunities of N-doped carbons as advanced oxygen electrocatalysts are highlighted.en_US
dc.relation.ispartofAdvanced Functional Materialsen_US
dc.rights© 2022 The Authors. Advanced Functional Materials published by Wiley-VCH GmbH. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.en_US
dc.titleNitrogen-rich carbonaceous materials for advanced oxygen electrocatalysis: synthesis, characterization, and activity of nitrogen sitesen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Materials Science and Engineeringen_US
dc.description.versionPublished versionen_US
dc.subject.keywordsCarbon Nanomaterialsen_US
dc.description.acknowledgementB.W., H.M., and D.M.M. contributed equally to this work. This work was supported by the Volkswagen Foundation (Freigeist Fellowship No. 89592). B.W. also acknowledges the funding by the CSC Fellowship. Open access funding enabled and organized by Projekt DEAL.en_US
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