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dc.contributor.authorLv, Jing-Jingen_US
dc.contributor.authorYin, Ruonanen_US
dc.contributor.authorZhou, Liminen_US
dc.contributor.authorLi, Junen_US
dc.contributor.authorKikas, Redduen_US
dc.contributor.authorXu, Tingen_US
dc.contributor.authorWang, Zheng-Junen_US
dc.contributor.authorJin, Huileen_US
dc.contributor.authorWang, Xinen_US
dc.contributor.authorWang, Shunen_US
dc.identifier.citationLv, J., Yin, R., Zhou, L., Li, J., Kikas, R., Xu, T., Wang, Z., Jin, H., Wang, X. & Wang, S. (2022). Microenvironment engineering for the electrocatalytic CO₂ reduction reaction. Angewandte Chemie (International Ed. in English), 61(39), e202207252-.
dc.description.abstractRather than just focusing on the catalyst itself in the electrocatalytic CO2 reduction reaction (eCO2 RR), as previously reviewed elsewhere, we herein extend the discussion to the special topic of the microenvironment around the electrocatalytic center and present a comprehensive overview of recent research progress. We categorize the microenvironment based on the components relevant to electrocatalytic active sites, i.e., the catalyst surface, substrate, co-reactants, electrolyte, membrane, and reactor. Supported by most of the reported articles, the relevant factors affecting the catalytic performance of eCO2 RR are then discussed in detail, and existing challenges and potential solutions are mentioned. Perspectives for the future research on eCO2 RR, including the integration of different microenvironment factors, the extension to industrial application by coupling with carbon capture and conversion, and separation of products, are also discussed.en_US
dc.relation.ispartofAngewandte Chemie (International ed. in English)en_US
dc.rights© 2022 Wiley-VCH GmbH. All rights reserved.en_US
dc.subjectEngineering::Chemical engineeringen_US
dc.titleMicroenvironment engineering for the electrocatalytic CO₂ reduction reactionen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Chemical and Biomedical Engineeringen_US
dc.subject.keywordsReduction Reactionen_US
dc.subject.keywordsMicroenvironment Engineeringen_US
dc.description.acknowledgementThis work was financially supported by the National Natural Science Foundation of China (51872209, 52072273), Zhejiang Provincial Special Support Program for High-level Talents (2019R52042), and Wenzhou basic scientific research project (No.2020G0076). J. J. Lv would like to acknowledge the Start-up Fund of Wenzhou University (QD2021152).en_US
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