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Title: Microenvironment engineering for the electrocatalytic CO₂ reduction reaction
Authors: Lv, Jing-Jing
Yin, Ruonan
Zhou, Limin
Li, Jun
Kikas, Reddu
Xu, Ting
Wang, Zheng-Jun
Jin, Huile
Wang, Xin
Wang, Shun
Keywords: Engineering::Chemical engineering
Issue Date: 2022
Source: Lv, J., Yin, R., Zhou, L., Li, J., Kikas, R., Xu, T., Wang, Z., Jin, H., Wang, X. & Wang, S. (2022). Microenvironment engineering for the electrocatalytic CO₂ reduction reaction. Angewandte Chemie (International Ed. in English), 61(39), e202207252-.
Journal: Angewandte Chemie (International ed. in English) 
Abstract: Rather than just focusing on the catalyst itself in the electrocatalytic CO2 reduction reaction (eCO2 RR), as previously reviewed elsewhere, we herein extend the discussion to the special topic of the microenvironment around the electrocatalytic center and present a comprehensive overview of recent research progress. We categorize the microenvironment based on the components relevant to electrocatalytic active sites, i.e., the catalyst surface, substrate, co-reactants, electrolyte, membrane, and reactor. Supported by most of the reported articles, the relevant factors affecting the catalytic performance of eCO2 RR are then discussed in detail, and existing challenges and potential solutions are mentioned. Perspectives for the future research on eCO2 RR, including the integration of different microenvironment factors, the extension to industrial application by coupling with carbon capture and conversion, and separation of products, are also discussed.
ISSN: 1433-7851
DOI: 10.1002/anie.202207252
Rights: © 2022 Wiley-VCH GmbH. All rights reserved.
Fulltext Permission: none
Fulltext Availability: No Fulltext
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