Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/164585
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dc.contributor.authorHuang, Tieqien_US
dc.contributor.authorXu, Kuien_US
dc.contributor.authorJia, Ningen_US
dc.contributor.authorYang, Lanen_US
dc.contributor.authorLiu, Hongtaoen_US
dc.contributor.authorZhu, Jixinen_US
dc.contributor.authorYan, Qingyuen_US
dc.date.accessioned2023-02-06T02:13:45Z-
dc.date.available2023-02-06T02:13:45Z-
dc.date.issued2023-
dc.identifier.citationHuang, T., Xu, K., Jia, N., Yang, L., Liu, H., Zhu, J. & Yan, Q. (2023). Intrinsic interfacial dynamic engineering of zincophilic microbrushes via regulating Zn deposition for highly reversible aqueous zinc ion battery. Advanced Materials, 35(5), 2205206-. https://dx.doi.org/10.1002/adma.202205206en_US
dc.identifier.issn0935-9648en_US
dc.identifier.urihttps://hdl.handle.net/10356/164585-
dc.description.abstractAqueous rechargeable zinc ion batteries are promising efficient energy storage systems due to remarkable safety and satisfactory capacity. However, zinc metal anode instability including dendrite growth and side reactions severely hinders widespread applications. Herein, zincophilic microbrushes have been in situ anchored on zinc plates through simple freeze-drying and mild reduction of graphene oxide, successfully overcoming these thorny issues. By introducing suitable oxygen-containing groups, the microbrushes exhibit a good affinity for zinc ions, thereby providing sufficient depositing sites, promoting zinc plating and stripping during cycling, and suppressing side reactions. The delicate zincophilic microbrushes can not only function as protective layer to guide the deposition of zinc ions, but also act as high-speed pathways to redistribute the zinc ion flux for rapid kinetics. Consequently, the microbrushes-covered zinc anode displays long lifespan and good durability, whenever in symmetric cell or full battery tests. This work paves a feasible bridge to design advanced aqueous anodes by architecting both structures and compositions of metal coverings.en_US
dc.description.sponsorshipMinistry of Education (MOE)en_US
dc.language.isoenen_US
dc.relation2020-T1-001-031en_US
dc.relation.ispartofAdvanced Materialsen_US
dc.rights© 2022 Wiley-VCH GmbH. All rights reserved.en_US
dc.subjectEngineering::Materialsen_US
dc.titleIntrinsic interfacial dynamic engineering of zincophilic microbrushes via regulating Zn deposition for highly reversible aqueous zinc ion batteryen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Materials Science and Engineeringen_US
dc.contributor.organizationInstitute of Materials Research and Engineering, A*STARen_US
dc.identifier.doi10.1002/adma.202205206-
dc.identifier.pmid36453716-
dc.identifier.scopus2-s2.0-85144200526-
dc.identifier.issue5en_US
dc.identifier.volume35en_US
dc.identifier.spage2205206en_US
dc.subject.keywordsAqueous Batteriesen_US
dc.subject.keywordsDendrite-Freeen_US
dc.description.acknowledgementThis work is financially supported by the National Natural Science Foundation of China (21905133, 52174284, 52172204, and 51872139) and MOE AcRF Tier 1 grant no. 2020-T1-001-031 (Singapore).en_US
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