Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/170530
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dc.contributor.authorLiu, Yongguien_US
dc.contributor.authorWang, Yanyanen_US
dc.contributor.authorWu, Xingxingen_US
dc.contributor.authorChi, Robin Yongguien_US
dc.date.accessioned2023-09-18T07:48:38Z-
dc.date.available2023-09-18T07:48:38Z-
dc.date.issued2023-
dc.identifier.citationLiu, Y., Wang, Y., Wu, X. & Chi, R. Y. (2023). Exploring molecular complexity by N-heterocyclic carbene organocatalysis: new activation and reaction diversity. The Chemical Record, 23(7), e202200219-. https://dx.doi.org/10.1002/tcr.202200219en_US
dc.identifier.issn1527-8999en_US
dc.identifier.urihttps://hdl.handle.net/10356/170530-
dc.description.abstractThe development of catalytic synthetic approaches towards molecular complexity from simple materials continues to be an ultimate goal in synthetic chemistry. Over the past decades, N-heterocyclic carbene (NHC) organocatalysis has been extensively investigated to provide opportunities for a vast number of novel chemical transformations. Various activation modes and reactive intermediates enabled by NHC small-molecule catalysts, such as Breslow intermediates, (homo)enolates, acyl azoliums and their derived unsaturated azoliums exhibit great potential in the construction of complicated skeletons. This personal account will summarize our group's recent work in the exploration of new activation modes of NHC catalysis towards molecular complexity with a focus on the development and applications of NHC to achieve diversity and enantioselectivity in the preparation of functional molecules.en_US
dc.description.sponsorshipMinistry of Education (MOE)en_US
dc.description.sponsorshipNanyang Technological Universityen_US
dc.description.sponsorshipNational Research Foundation (NRF)en_US
dc.language.isoenen_US
dc.relationNRF-NRFI2016-06en_US
dc.relationNRF-CRP22-2019-0002en_US
dc.relationRG7/20en_US
dc.relationRG5/19en_US
dc.relationMOE2019-T2-2-117en_US
dc.relationMOE2018-T3-1-003en_US
dc.relation.ispartofThe Chemical Recorden_US
dc.rights© 2022 The Chemical Society of Japan & Wiley-VCH GmbH. All rights reserved.en_US
dc.subjectScience::Chemistryen_US
dc.titleExploring molecular complexity by N-heterocyclic carbene organocatalysis: new activation and reaction diversityen_US
dc.typeJournal Articleen
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen_US
dc.identifier.doi10.1002/tcr.202200219-
dc.identifier.pmid36344433-
dc.identifier.scopus2-s2.0-85141446959-
dc.identifier.issue7en_US
dc.identifier.volume23en_US
dc.identifier.spagee202200219en_US
dc.subject.keywordsOrganocatalysisen_US
dc.subject.keywordsAsymmetric Catalysisen_US
dc.description.acknowledgementWe acknowledge financial support from the National Natural Science Foundation of China (21772029, 21801051, 21961006, 22001173), National Natural Science Fund for Excellent Young Scientists Fund Program (Overseas), The 10 Talent Plan (Shicengci) of Guizhou Province ([2016]5649), the Science and Technology Department of Guizhou Province ([2019]1020, Qianke‐hejichu‐ZK[2021]Key033), the starting grant of Guizhou University [(2022)47)], Frontiers Science Center for Asymmetric Synthesis and Medicinal Molecules, Department of Education, Guizhou Province [Qianjiaohe KY (2020)004], the Basic and Applied Research Foundation of Guangdong Province (2019A1515110906), the Guizhou Province First‐Class Disci‐plines Project [(Yiliu Xueke Jianshe Xiangmu)‐GNYL(2017)008], Guizhou University of Traditional Chinese Medicine, and Guizhou University (China). Singapore National Research Foundation under its NRF Investigatorship (NRF‐NRFI2016‐06) and Competitive Research Program (NRF‐CRP22‐2019‐0002); the Ministry of Education, Singapore, under its MOE AcRF Tier 1 Award (RG7/20, RG5/19), MOE AcRF Tier 2 (MOE2019‐T2‐2‐117), MOE AcRF Tier 3 Award (MOE2018‐T3‐1‐003); Nanyang Research Award Grant, Chair Professorship Grant, Nanyang Technological University.en_US
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