Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/171427
Title: Random organization and non-equilibrium hyperuniform fluids on a sphere
Authors: Lei, Yusheng
Zheng, Ning
Ni, Ran
Keywords: Science::Chemistry
Issue Date: 2023
Source: Lei, Y., Zheng, N. & Ni, R. (2023). Random organization and non-equilibrium hyperuniform fluids on a sphere. Journal of Chemical Physics, 159(8), 081101-1-081101-6. https://dx.doi.org/10.1063/5.0165527
Project: MOE2019-T2-2-010 
Journal: Journal of Chemical Physics 
Abstract: Randomly organizing hyperuniform fluid induced by reciprocal activation is a non-equilibrium fluid with vanishing density fluctuations at large length scales such as crystals. Here, we extend this new state of matter to a closed manifold, namely a spherical surface. We find that the random organization on a spherical surface behaves similar to that in two dimensional Euclidean space, and the absorbing transition on a sphere also belongs to the conserved directed percolation universality class. Moreover, the reciprocal activation can also induce a non-equilibrium hyperuniform fluid on a sphere. The spherical structure factor at the absorbing transition and the non-equilibrium hyperuniform fluid phases are scaled as S(l → 0) ∼ (l/R)0.45 and S(l → 0) ∼ l(l + 1)/R2, respectively, which are both hyperuniform according to the definition of hyperuniformity on a sphere with l, the wave number, and R, the radius of the spherical surface. We also consider the impact of inertia in realistic hyperuniform fluids, and it is found only by adding an extra length-scale, above which hyperuniform scaling appears. Our finding suggests a new method for creating non-equilibrium hyperuniform fluids on closed manifolds to avoid boundary effects.
URI: https://hdl.handle.net/10356/171427
ISSN: 0021-9606
DOI: 10.1063/5.0165527
Schools: School of Chemistry, Chemical Engineering and Biotechnology 
Rights: © 2023 Author(s). Published under an exclusive license by AIP Publishing. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1063/5.0165527
Fulltext Permission: open
Fulltext Availability: With Fulltext
Appears in Collections:CCEB Journal Articles

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