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https://hdl.handle.net/10356/173778
Title: | Contracted description of driven degenerate multilevel quantum systems | Authors: | Xu, Xiangyu Sun, Kewei Gelin, Maxim F. Zhao, Yang |
Keywords: | Engineering | Issue Date: | 2023 | Source: | Xu, X., Sun, K., Gelin, M. F. & Zhao, Y. (2023). Contracted description of driven degenerate multilevel quantum systems. Journal of Chemical Physics, 159(22). https://dx.doi.org/10.1063/5.0178460 | Project: | RG87/20 | Journal: | Journal of Chemical Physics | Abstract: | We formulate a contraction theorem that maps quantum dynamics of a multilevel degenerate system (DS) driven by a time-dependent external field to the dynamics of the corresponding contracted non-degenerate system (CNS) of lower dimension, provided transitions between each pair of degenerate levels in the DS have identical transition dipole moments. The theorem is valid for an external field of any strength and shape, with and without rotating wave approximation in the system-field interaction. It establishes explicit relations between DS and CNS observables, significantly simplifies numerical calculations, and clarifies physical origins of the field-induced DS dynamics. | URI: | https://hdl.handle.net/10356/173778 | ISSN: | 0021-9606 | DOI: | 10.1063/5.0178460 | Schools: | School of Materials Science and Engineering | Rights: | © 2023 Author(s). Published under an exclusive license by AIP Publishing. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1063/5.0178460 | Fulltext Permission: | open | Fulltext Availability: | With Fulltext |
Appears in Collections: | MSE Journal Articles |
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