Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/82240
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dc.contributor.authorZhang, Zhengyangen
dc.contributor.authorWells, Kym L.en
dc.contributor.authorSeidel, Marco T.en
dc.contributor.authorTan, Howe-Siangen
dc.date.accessioned2016-01-29T06:34:09Zen
dc.date.accessioned2019-12-06T14:51:32Z-
dc.date.available2016-01-29T06:34:09Zen
dc.date.available2019-12-06T14:51:32Z-
dc.date.issued2013en
dc.identifier.citationZhang, Z., Wells, K. L., Seidel, M. T., & Tan, H.-S. (2013). Fifth-Order Three-Dimensional Electronic Spectroscopy Using a Pump–Probe Configuration. The Journal of Physical Chemistry B, 117(49), 15369-15385.en
dc.identifier.issn1520-6106en
dc.identifier.urihttps://hdl.handle.net/10356/82240-
dc.description.abstractWe present the theoretical details and experimental demonstration of fifth-order three-dimensional (3D) electronic spectroscopy using a pump–probe beam geometry. This is achieved using a pulse shaper and appropriate phase cycling schemes. We show how 8-step and 27-step phase cycling schemes can measure purely absorptive 3D spectra as well as 3D spectra for the individual fifth-order processes that contribute to the purely absorptive spectrum. 3D spectra as a function of two separate controllable waiting time periods can be obtained. The peak shapes and positions of the peaks in the experimental measurement correspond well to theory.en
dc.description.sponsorshipNRF (Natl Research Foundation, S’pore)en
dc.description.sponsorshipASTAR (Agency for Sci., Tech. and Research, S’pore)en
dc.format.extent53 p.en
dc.language.isoenen
dc.relation.ispartofseriesThe Journal of Physical Chemistry Ben
dc.rights© 2013 American Chemical Society. This is the author created version of a work that has been peer reviewed and accepted for publication by The Journal of Physical Chemistry B, American Chemical Society. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [http://dx.doi.org/10.1021/jp4046403].en
dc.subjectChemistry and Biological Chemistryen
dc.titleFifth-Order Three-Dimensional Electronic Spectroscopy Using a Pump–Probe Configurationen
dc.typeJournal Articleen
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen
dc.identifier.doi10.1021/jp4046403en
dc.description.versionAccepted versionen
item.grantfulltextopen-
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