Please use this identifier to cite or link to this item:
Full metadata record
DC FieldValueLanguage
dc.contributor.authorZhang, Zhengyangen
dc.contributor.authorWells, Kym L.en
dc.contributor.authorSeidel, Marco T.en
dc.contributor.authorTan, Howe-Siangen
dc.identifier.citationZhang, Z., Wells, K. L., Seidel, M. T., & Tan, H.-S. (2013). Fifth-Order Three-Dimensional Electronic Spectroscopy Using a Pump–Probe Configuration. The Journal of Physical Chemistry B, 117(49), 15369-15385.en
dc.description.abstractWe present the theoretical details and experimental demonstration of fifth-order three-dimensional (3D) electronic spectroscopy using a pump–probe beam geometry. This is achieved using a pulse shaper and appropriate phase cycling schemes. We show how 8-step and 27-step phase cycling schemes can measure purely absorptive 3D spectra as well as 3D spectra for the individual fifth-order processes that contribute to the purely absorptive spectrum. 3D spectra as a function of two separate controllable waiting time periods can be obtained. The peak shapes and positions of the peaks in the experimental measurement correspond well to theory.en
dc.description.sponsorshipNRF (Natl Research Foundation, S’pore)en
dc.description.sponsorshipASTAR (Agency for Sci., Tech. and Research, S’pore)en
dc.format.extent53 p.en
dc.relation.ispartofseriesThe Journal of Physical Chemistry Ben
dc.rights© 2013 American Chemical Society. This is the author created version of a work that has been peer reviewed and accepted for publication by The Journal of Physical Chemistry B, American Chemical Society. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [].en
dc.subjectChemistry and Biological Chemistryen
dc.titleFifth-Order Three-Dimensional Electronic Spectroscopy Using a Pump–Probe Configurationen
dc.typeJournal Articleen
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen
dc.description.versionAccepted versionen
item.fulltextWith Fulltext-
Appears in Collections:SPMS Journal Articles
Files in This Item:
File Description SizeFormat 
Fifth-Order Three-Dimensional Electronic Spectroscopy Using a Pump-Probe Configuration.pdf5.1 MBAdobe PDFThumbnail

Citations 10

Updated on Jun 9, 2024

Web of ScienceTM
Citations 20

Updated on Oct 28, 2023

Page view(s) 50

Updated on Jun 11, 2024

Download(s) 10

Updated on Jun 11, 2024

Google ScholarTM




Items in DR-NTU are protected by copyright, with all rights reserved, unless otherwise indicated.