Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/82766
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dc.contributor.authorOng, S. W. Danielen
dc.contributor.authorLin, Jianyien
dc.contributor.authorSeebauer, Edmund G.en
dc.date.accessioned2016-03-29T08:22:57Zen
dc.date.accessioned2019-12-06T15:05:08Z-
dc.date.available2016-03-29T08:22:57Zen
dc.date.available2019-12-06T15:05:08Z-
dc.date.issued2015en
dc.identifier.citationOng, S. W. D., Lin, J., & Seebauer, E. G. (2015). Control of methylene blue photo-oxidation rate over polycrystalline anatase TiO2 thin films via carrier concentration. The Journal of Physical Chemistry C, 119(21), 11662-11671.en
dc.identifier.issn1932-7447en
dc.identifier.urihttps://hdl.handle.net/10356/82766-
dc.description.abstractReaction rates on photocatalytic surfaces would often benefit greatly if minority photocar-riers could be driven more efficiently to the surface through the manipulation of electric fields within the semiconductor. Such field-induced manipulation of photocurrent is commonplace in conventional optoe-lectronics, but translation to photochemistry and photoelectrochemistry has lagged. The present work demonstrates quantitatively that manipulation of the spatial extent of band bending via background carrier concentration can increase photoreaction rates by a factor of five or more in the case of methylene blue photodegradation over thin-film polycrystalline anatase TiO2. A quantitative photocurrent model fits closely to experimental rate data with no adjustable parameters.en
dc.description.sponsorshipASTAR (Agency for Sci., Tech. and Research, S’pore)en
dc.format.extent32 p.en
dc.language.isoenen
dc.relation.ispartofseriesThe Journal of Physical Chemistry Cen
dc.rights© 2015 American Chemical Society. This is the author created version of a work that has been peer reviewed and accepted for publication by Journal of Physical Chemistry C, American Chemical Society. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [http://dx.doi.org/10.1021/acs.jpcc.5b01852].en
dc.subjectBand-bendingen
dc.subjectPhotocatalysisen
dc.subjectTiO2en
dc.subjectfilmen
dc.subjectDefect engineeringen
dc.subjectBand engineeringen
dc.titleControl of Methylene Blue Photo-Oxidation Rate over Polycrystalline Anatase TiO2 Thin Films via Carrier Concentrationen
dc.typeJournal Articleen
dc.contributor.researchEnergy Research Institute @ NTU (ERI@N)en
dc.identifier.doi10.1021/acs.jpcc.5b01852en
dc.description.versionAccepted versionen
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item.grantfulltextopen-
Appears in Collections:ERI@N Journal Articles

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