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https://hdl.handle.net/10356/83277
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DC Field | Value | Language |
---|---|---|
dc.contributor.author | Barát, Viktor | en |
dc.contributor.author | Csókás, Dániel | en |
dc.contributor.author | Bates, Roderick Wayland | en |
dc.date.accessioned | 2019-10-03T02:49:29Z | en |
dc.date.accessioned | 2019-12-06T15:19:01Z | - |
dc.date.available | 2019-10-03T02:49:29Z | en |
dc.date.available | 2019-12-06T15:19:01Z | - |
dc.date.issued | 2018 | en |
dc.identifier.citation | Barát, V., Csókás, D., & Bates, R. W. (2018). Synthesis of (−)-cytisine Using a 6- endo aza-Michael addition. The Journal of Organic Chemistry, 83(16), 9088-9095. doi:10.1021/acs.joc.8b01156 | en |
dc.identifier.issn | 0022-3263 | en |
dc.identifier.uri | https://hdl.handle.net/10356/83277 | - |
dc.description.abstract | An asymmetric synthesis of (-)-cytisine has been achieved. The piperidine C-ring was formed using a stereodivergent intramolecular 6-endo aza-Michael addition. The B-ring was established by intramolecular pyridine N-alkylation. The absolute stereochemistry was established by an Evans acyl oxazolidinone enolate alkylation reaction that proceeded with an unexpected stereochemical outcome due to participation of the pyridine nitrogen lone pair. | en |
dc.description.sponsorship | MOE (Min. of Education, S’pore) | en |
dc.format.extent | 29 p. | en |
dc.language.iso | en | en |
dc.relation.ispartofseries | The Journal of Organic Chemistry | en |
dc.rights | This document is the Accepted Manuscript version of a Published Work that appeared in final form in The Journal of Organic Chemistry, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.joc.8b01156 | en |
dc.subject | Chemistry | en |
dc.subject | Science::Chemistry::Organic chemistry | en |
dc.subject | Stereochemistry | en |
dc.title | Synthesis of (−)-cytisine using a 6-endo aza-Michael addition | en |
dc.type | Journal Article | en |
dc.contributor.school | School of Physical and Mathematical Sciences | en |
dc.identifier.doi | 10.1021/acs.joc.8b01156 | en |
dc.description.version | Accepted version | en |
item.grantfulltext | open | - |
item.fulltext | With Fulltext | - |
Appears in Collections: | SPMS Journal Articles |
Files in This Item:
File | Description | Size | Format | |
---|---|---|---|---|
Cytisine JOC revised.pdf | accepted manuscript | 6.37 MB | Adobe PDF | ![]() View/Open |
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