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dc.contributor.authorZhang, Yanyanen
dc.contributor.authorRui, Xianhongen
dc.contributor.authorTang, Yuxinen
dc.contributor.authorLiu, Yaqingen
dc.contributor.authorWei, Jiaqien
dc.contributor.authorChen, Shien
dc.contributor.authorLeow, Wan Ruen
dc.contributor.authorLi, Wenlongen
dc.contributor.authorLiu, Yuanjunen
dc.contributor.authorDeng, Jiyangen
dc.contributor.authorMa, Bingen
dc.contributor.authorYan, Qingyuen
dc.contributor.authorChen, Xiaodongen
dc.identifier.citationZhang, Y., Rui, X., Tang, Y., Liu, Y., Wei, J., Chen, S., et al. (2016). Wet-Chemical Processing of Phosphorus Composite Nanosheets for High-Rate and High-Capacity Lithium-Ion Batteries. Advanced Energy Materials, 6(10), 1502409-.en
dc.description.abstractPhosphorus-based materials are promising for high-performance lithium-ion battery (LIB) applications due to their high theoretical specific capacity. Currently, the existing physical methods render great difficulty toward rational engineering on the nanostructural phosphorus or its composites, thus limiting its high-rate LIB applications. For the first time, a sublimation-induced synthesis of phosphorus-based composite nanosheets by a chemistry-based solvothermal reaction is reported. Its formation mechanism involves solid–vapor–solid transformation driven by continuous vaporization–condensation process, as well as subsequent bottom-up assembly growth. The proof-of-concept LIBs composed of the phosphorus-based nanosheets achieve a high capacity of 630 mAh g−1 at an ultrahigh current density of 20 A g−1, which is attributed to efficient lithium-ion diffusion and electron transfer. Such simple sublimation-induced transformation opens up new prospects for rational engineering of phosphorus-based materials for enhancing electrochemical performance.en
dc.description.sponsorshipNRF (Natl Research Foundation, S’pore)en
dc.description.sponsorshipMOE (Min. of Education, S’pore)en
dc.format.extent23 p.en
dc.relation.ispartofseriesAdvanced Energy Materialsen
dc.rights© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. This is the author created version of a work that has been peer reviewed and accepted for publication by Advanced Energy Materials, WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [].en
dc.subjectLithium-ion batteriesen
dc.subjectPhosphorus composite nanosheetsen
dc.titleWet-Chemical Processing of Phosphorus Composite Nanosheets for High-Rate and High-Capacity Lithium-Ion Batteriesen
dc.typeJournal Articleen
dc.contributor.schoolSchool of Materials Science & Engineeringen
dc.contributor.schoolSchool of Physical and Mathematical Sciencesen
dc.description.versionAccepted versionen
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