Please use this identifier to cite or link to this item: https://hdl.handle.net/10356/88633
Title: Polymer-fluorinated silica composite hollow fiber membranes for the recovery of biogas dissolved in anaerobic effluent
Authors: Wongchitphimon, Sunee
Rongwong, Wichitpan
Chuah, Chong Yang
Wang, Rong
Bae, Tae-Hyun
Keywords: Dissolved Methane Recovery
Biogas
Issue Date: 2017
Source: Wongchitphimon, S., Rongwong, W., Chuah, C. Y., Wang, R., & Bae, T.-H. (2017). Polymer-fluorinated silica composite hollow fiber membranes for the recovery of biogas dissolved in anaerobic effluent. Journal of Membrane Science, 540, 146-154.
Series/Report no.: Journal of Membrane Science
Abstract: In this study, polymer-fluorinated silica composite hollow fiber membranes were fabricated and applied to a membrane contactor system for the recovery of methane dissolved in the anaerobic effluent. Such composite membranes allowed us to tailor the physical property such as porosity and mechanical strength and the surface hydrophobicity in separated processes. To develop the composite membranes, porous hollow fiber substrates were first fabricated with Matrimid®, a commercial polyimide. Subsequently, fluorinated silica particles were synthesized and anchored on the substrates via a strong covalent bonding. Due to the high porosity as well as the high hydrophobicity, our membrane showed an outstanding performance for the recovery of CH4 in the membrane contactor, such that the CH4 flux reached 2900 mg CH4/m2–h at the liquid velocity of 0.42 m/s at which the liquid phase still controlled the overall mass transfer. The composite membrane prepared in this work also showed a much better performance in the CH4 recovery than a commercial polypropylene membrane made for degasification of water. In addition, a long-term test with tap water saturated with the model biogas made up of 60:40 CH4/CO2 mixture demonstrated that our membrane can be stably operated for more than 300 h without experiencing pore wetting problem.
URI: https://hdl.handle.net/10356/88633
http://hdl.handle.net/10220/44702
ISSN: 0376-7388
DOI: 10.1016/j.memsci.2017.06.050
Rights: © 2017 Elsevier B.V. This is the author created version of a work that has been peer reviewed and accepted for publication by Journal of Membrane Science, Elsevier B.V. It incorporates referee’s comments but changes resulting from the publishing process, such as copyediting, structural formatting, may not be reflected in this document. The published version is available at: [http://dx.doi.org/10.1016/j.memsci.2017.06.050].
Fulltext Permission: open
Fulltext Availability: With Fulltext
Appears in Collections:CEE Journal Articles

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